<p>The decommissioning of nuclear facilities generates metallic waste containing difficult-to-measure radionuclides (DTMs), whose accurate quantification requires destructive analyses to support effective waste management. This review highlights recent advances in dissolution, radiochemical separation, and high-sensitivity detection for activation products, long-lived fission products, and exotic DTMs. Remaining challenges include sampling, matrix effects, and the lack of reference materials, highlighting the need for methodological standardization and regulatory harmonization.</p>

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Toward sustainable nuclear material management: a review of destructive methods for quantifying difficult-to-measure radionuclides in metallic waste

  • Lu Liu,
  • Paul Dutheil,
  • Eya Abed,
  • Mathurin Robin,
  • Anne-Laure Nivesse,
  • Gilles Montavon,
  • Steffen Happel,
  • Maria Boltoeva,
  • Tomo Suzuki-Muresan

摘要

The decommissioning of nuclear facilities generates metallic waste containing difficult-to-measure radionuclides (DTMs), whose accurate quantification requires destructive analyses to support effective waste management. This review highlights recent advances in dissolution, radiochemical separation, and high-sensitivity detection for activation products, long-lived fission products, and exotic DTMs. Remaining challenges include sampling, matrix effects, and the lack of reference materials, highlighting the need for methodological standardization and regulatory harmonization.