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<p>Advanced Oxidation Processes (AOPs) are promising for treating persistent pollutants, yet challenges arise due to the step-wise oxidants activation process, which traditional single-active-center catalysts struggle to facilitate effectively. Recently, dual-active-center catalysts have emerged as a solution by enabling synergistic reactions. This review covers advances in these catalysts, their co-catalytic mechanisms, and applications in electro-Fenton, photocatalytic, peroxymonosulfate-, and pollutant-as-electron-donor based Fenton-like processes, along with active site design considerations and future challenges.</p>

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Site-designed dual-active-center catalysts for co-catalysis in advanced oxidation processes

  • 期刊论文

  • 出版模式：

    开放获取

  • 发表日期：

    2025年1月7日

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  • Wenxin Sun,
  • Guoshuai Liu,
  • Hua Zou,
  • Shaobin Wang,
  • Xiaoguang Duan

摘要

Advanced Oxidation Processes (AOPs) are promising for treating persistent pollutants, yet challenges arise due to the step-wise oxidants activation process, which traditional single-active-center catalysts struggle to facilitate effectively. Recently, dual-active-center catalysts have emerged as a solution by enabling synergistic reactions. This review covers advances in these catalysts, their co-catalytic mechanisms, and applications in electro-Fenton, photocatalytic, peroxymonosulfate-, and pollutant-as-electron-donor based Fenton-like processes, along with active site design considerations and future challenges.