<p>Interfaces between correlated oxides and strong spin–orbit coupled materials provide a fertile platform for emergent quantum phases, yet controlling these phases through interfacial magnetic reconstruction remains a major challenge. Here, we observe emergent metallicity in ultrathin SrIrO<sub>3</sub>/SrRuO<sub>3</sub> heterostructures formed from insulating constituent layers, and this transition is closely associated with interfacial magnetic reconstruction. Combining transport, magnetometry, and angle-resolved photoemission spectroscopy, supported by first-principles calculations, we show that finite spectral weight at the Fermi level and ferromagnetic signatures emerge in the heterostructures. Our calculations further suggest that a staggered Dzyaloshinskii–Moriya interaction at the interface favors ferromagnetic order in SrRuO₃ and collinear antiferromagnetism in SrIrO₃, relative to the collinear and noncollinear antiferromagnetism in isolated ultrathin SrRuO₃ and SrIrO₃, respectively, providing a possible microscopic framework for the coupled magnetic and electronic reconstruction. Our findings identify interfacial magnetic interactions as a powerful tuning parameter for controlling correlated electronic phases in spin-orbit-coupled oxides, opening pathways toward the design of emergent quantum and topological states.</p>

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Interfacial magnetic reconstruction and emergent metallicity in oxide heterostructures

  • Zengxing Lu,
  • Jiatai Feng,
  • Xuan Zheng,
  • You-Guo Shi,
  • Run-Wei Li,
  • Nicholas C. Plumb,
  • Carmine Autieri,
  • Mario Cuoco,
  • Zhiming Wang,
  • Milan Radovic

摘要

Interfaces between correlated oxides and strong spin–orbit coupled materials provide a fertile platform for emergent quantum phases, yet controlling these phases through interfacial magnetic reconstruction remains a major challenge. Here, we observe emergent metallicity in ultrathin SrIrO3/SrRuO3 heterostructures formed from insulating constituent layers, and this transition is closely associated with interfacial magnetic reconstruction. Combining transport, magnetometry, and angle-resolved photoemission spectroscopy, supported by first-principles calculations, we show that finite spectral weight at the Fermi level and ferromagnetic signatures emerge in the heterostructures. Our calculations further suggest that a staggered Dzyaloshinskii–Moriya interaction at the interface favors ferromagnetic order in SrRuO₃ and collinear antiferromagnetism in SrIrO₃, relative to the collinear and noncollinear antiferromagnetism in isolated ultrathin SrRuO₃ and SrIrO₃, respectively, providing a possible microscopic framework for the coupled magnetic and electronic reconstruction. Our findings identify interfacial magnetic interactions as a powerful tuning parameter for controlling correlated electronic phases in spin-orbit-coupled oxides, opening pathways toward the design of emergent quantum and topological states.