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<p>Van der Waals-interfacial heat transfer is a key element in thermal problems in atomic-scale devices including quantum computing devices, solid-state batteries, and solar power generation devices. However, its characterization remains challenging due to the lack of atomic-scale measurement technologies. Here, we use custom-fabricated scanning probes with embedded highly precise thermometers and an atomic milling technique to simultaneously measure heat transfer and the van der Waals interactions at atomic contacts. Experimental results indicate the transformation of the heat transfer mechanism with increasing van der Waals atomic interactions. We identify the transition from single-atomic to multi-atomic channel mediated heat transfer through analysis using the Rabinovich model together with molecular dynamics simulations. Additionally, we confirm the same transition mechanism in various van der Waals interfaces and identify differences in their interfacial regions. This work provides an experimental framework and insights for understanding van der Waals-interfacial heat transfer.</p>

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Atomic heat transfer in nanoscale contacts mediated by van der Waals interactions

  • 期刊论文

  • 出版模式：

    开放获取

  • 发表日期：

    2026年5月27日

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  • Seunghoe Koo,
  • Jaehee Park,
  • Junki Jung,
  • Hyo Jae Yoon,
  • Seungha Shin,
  • Minsub Han,
  • Kyeongtae Kim

摘要

Van der Waals-interfacial heat transfer is a key element in thermal problems in atomic-scale devices including quantum computing devices, solid-state batteries, and solar power generation devices. However, its characterization remains challenging due to the lack of atomic-scale measurement technologies. Here, we use custom-fabricated scanning probes with embedded highly precise thermometers and an atomic milling technique to simultaneously measure heat transfer and the van der Waals interactions at atomic contacts. Experimental results indicate the transformation of the heat transfer mechanism with increasing van der Waals atomic interactions. We identify the transition from single-atomic to multi-atomic channel mediated heat transfer through analysis using the Rabinovich model together with molecular dynamics simulations. Additionally, we confirm the same transition mechanism in various van der Waals interfaces and identify differences in their interfacial regions. This work provides an experimental framework and insights for understanding van der Waals-interfacial heat transfer.