<p>Unconventional charge- and spin-density-wave states are commonly observed in bilayer nickelates, drawing considerable attention due to their proximity to high-transition temperature (<InlineEquation ID="IEq1"> <EquationSource Format="TEX">\({T}_{{\rm{c}}}\)</EquationSource> <EquationSource Format="MATHML"><math> <msub> <mrow> <mi>T</mi> </mrow> <mrow> <mi mathvariant="normal">c</mi> </mrow> </msub> </math></EquationSource> </InlineEquation>) superconductivity. However, the nature and origin of these density waves remain poorly understood. Experiments show that the charge-density-wave and spin-density-wave transition temperatures are closely related but distinct, while mean-field-type analyses typically have yielded only a simple spin-density-wave phase. To resolve this key problem, this paper demonstrates that sizeable charge-density-wave instabilities emerge in proportion to spin-density-wave instabilities in La<sub>3</sub>Ni<sub>2</sub>O<sub>7</sub> due to the paramagnon-interference mechanism, which captures electron correlations beyond mean-field theories. Therefore, (i) the experimental charge- and spin-density-wave coexisting state is naturally explained, and (ii) charge- and spin-density-wave fluctuations cooperatively drive high-<InlineEquation ID="IEq2"> <EquationSource Format="TEX">\({T}_{{\rm{c}}}\)</EquationSource> <EquationSource Format="MATHML"><math> <msub> <mrow> <mi>T</mi> </mrow> <mrow> <mi mathvariant="normal">c</mi> </mrow> </msub> </math></EquationSource> </InlineEquation> superconductivity. Furthermore, the predicted s-wave superconducting state is robust against the inner-apical oxygen vacancies. We find that the coexistence of charge- and spin-fluctuations is essential in bilayer nickelates, with both playing a cooperative role in mediating high-<InlineEquation ID="IEq3"> <EquationSource Format="TEX">\({T}_{{\rm{c}}}\)</EquationSource> <EquationSource Format="MATHML"><math> <msub> <mrow> <mi>T</mi> </mrow> <mrow> <mi mathvariant="normal">c</mi> </mrow> </msub> </math></EquationSource> </InlineEquation> superconductivity.</p>

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Unified mechanism of charge-density-wave and high-Tc superconductivity protected from oxygen vacancies in bilayer nickelates

  • Daisuke Inoue,
  • Youichi Yamakawa,
  • Seiichiro Onari,
  • Hiroshi Kontani

摘要

Unconventional charge- and spin-density-wave states are commonly observed in bilayer nickelates, drawing considerable attention due to their proximity to high-transition temperature ( \({T}_{{\rm{c}}}\) T c ) superconductivity. However, the nature and origin of these density waves remain poorly understood. Experiments show that the charge-density-wave and spin-density-wave transition temperatures are closely related but distinct, while mean-field-type analyses typically have yielded only a simple spin-density-wave phase. To resolve this key problem, this paper demonstrates that sizeable charge-density-wave instabilities emerge in proportion to spin-density-wave instabilities in La3Ni2O7 due to the paramagnon-interference mechanism, which captures electron correlations beyond mean-field theories. Therefore, (i) the experimental charge- and spin-density-wave coexisting state is naturally explained, and (ii) charge- and spin-density-wave fluctuations cooperatively drive high- \({T}_{{\rm{c}}}\) T c superconductivity. Furthermore, the predicted s-wave superconducting state is robust against the inner-apical oxygen vacancies. We find that the coexistence of charge- and spin-fluctuations is essential in bilayer nickelates, with both playing a cooperative role in mediating high- \({T}_{{\rm{c}}}\) T c superconductivity.