<p>Dust aerosols constitute a major component of shortwave-absorbing aerosols, with absorption uncertainties predominantly associated with mineral composition variations. To address this, we analyzed 22 East Asian dust (EAD) samples and derived a revised imaginary part of the complex refractive index (<InlineEquation ID="IEq1"> <EquationSource Format="TEX">\(k\)</EquationSource> <EquationSource Format="MATHML"><math> <mi>k</mi> </math></EquationSource> </InlineEquation>), with a range spanning from <InlineEquation ID="IEq2"> <EquationSource Format="TEX">\(2.26\times {10}^{-4}\)</EquationSource> <EquationSource Format="MATHML"><math> <mrow> <mn>2.26</mn> <mo>×</mo> <msup> <mrow> <mn>10</mn> </mrow> <mrow> <mo>−</mo> <mn>4</mn> </mrow> </msup> </mrow> </math></EquationSource> </InlineEquation>–<InlineEquation ID="IEq3"> <EquationSource Format="TEX">\(8.37\times {10}^{-4}\)</EquationSource> <EquationSource Format="MATHML"><math> <mrow> <mn>8.37</mn> <mo>×</mo> <msup> <mrow> <mn>10</mn> </mrow> <mrow> <mo>−</mo> <mn>4</mn> </mrow> </msup> </mrow> </math></EquationSource> </InlineEquation> in 0.3–1 <i>μ</i>m, which is significantly lower than the Optical Properties of Aerosols and Clouds (OPAC) and the values commonly used in research on East Asian. The improved optical parameters applied to CAS-ESM2 for spring dust simulations have been shown to reduce single scattering albedo (SSA) bias from 15% to 2% and absorption aerosol optical depth (AAOD) overestimation from +5.2% to −1.7%. The modified scheme reduces atmospheric absorption by 79.5% (−7.61 W/m<sup>2</sup>) and reverses the top of atmospheric shortwave radiation effect to −3.80 W/m<sup>2</sup>. This outcome revealed that dust absorption in East Asia is weak and the climate impact is significantly different from previous assessments.</p>

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Weaker absorption of Asian dust than previously estimated based on observation-constrained simulation

  • Youjia Yuan,
  • Hao Wang,
  • Chenglai Wu,
  • Tafeng Hu,
  • Feng Wu,
  • Daizhou Zhang,
  • Junji Cao

摘要

Dust aerosols constitute a major component of shortwave-absorbing aerosols, with absorption uncertainties predominantly associated with mineral composition variations. To address this, we analyzed 22 East Asian dust (EAD) samples and derived a revised imaginary part of the complex refractive index ( \(k\) k ), with a range spanning from \(2.26\times {10}^{-4}\) 2.26 × 10 4 \(8.37\times {10}^{-4}\) 8.37 × 10 4 in 0.3–1 μm, which is significantly lower than the Optical Properties of Aerosols and Clouds (OPAC) and the values commonly used in research on East Asian. The improved optical parameters applied to CAS-ESM2 for spring dust simulations have been shown to reduce single scattering albedo (SSA) bias from 15% to 2% and absorption aerosol optical depth (AAOD) overestimation from +5.2% to −1.7%. The modified scheme reduces atmospheric absorption by 79.5% (−7.61 W/m2) and reverses the top of atmospheric shortwave radiation effect to −3.80 W/m2. This outcome revealed that dust absorption in East Asia is weak and the climate impact is significantly different from previous assessments.