Scholarlink

<p>This work presents a novel approach for high-efficiency modeling of composite halide perovskite solar cells using the Fractional Differential Quadrature (FDQ) method. The FDQ method is applied to solve the governing equations derived from continuity and Poisson equations describing charge transport in a specific perovskite structure (PCBM/CH3NH3GeI3/CuI) solar cell. Our simulations demonstrate high accuracy with an error margin of 10⁻⁸ compared to experimental data and significant computational efficiency compared to other experimental and numerical methods. A detailed parametric study investigated the influence of temperature, layer thickness, charge carrier mobilities, and bandgaps on key performance indicators, including short-circuit current (Jsc), open-circuit voltage (Voc), fill factor (FF), and power conversion efficiency (PCE). Key findings include a maximum Jsc with a 300&#xa0;nm increase in HTL thickness, a 7.5% decrease in PCE with a 50&#xa0;nm increase in ETL thickness. These results provide valuable insights for optimizing the design and fabrication of high-performance composite halide perovskite solar cells and demonstrate the potential of the FDQ method as a powerful tool for device modeling and optimization.</p>

错误：搜索内容不能为空，请输入英文关键词
错误：关键词超出字数限制，请精简
高级检索

Fractional differential quadrature method for modeling composite halide perovskite solar cells

  • 期刊论文

  • 出版模式：

    开放获取

  • 发表日期：

    2025年8月22日

查看全文
  • Ehab M. Almetwally,
  • Ola Ragb,
  • Mohamed Salah,
  • Mokhtar Mohamed

摘要

This work presents a novel approach for high-efficiency modeling of composite halide perovskite solar cells using the Fractional Differential Quadrature (FDQ) method. The FDQ method is applied to solve the governing equations derived from continuity and Poisson equations describing charge transport in a specific perovskite structure (PCBM/CH3NH3GeI3/CuI) solar cell. Our simulations demonstrate high accuracy with an error margin of 10⁻⁸ compared to experimental data and significant computational efficiency compared to other experimental and numerical methods. A detailed parametric study investigated the influence of temperature, layer thickness, charge carrier mobilities, and bandgaps on key performance indicators, including short-circuit current (Jsc), open-circuit voltage (Voc), fill factor (FF), and power conversion efficiency (PCE). Key findings include a maximum Jsc with a 300 nm increase in HTL thickness, a 7.5% decrease in PCE with a 50 nm increase in ETL thickness. These results provide valuable insights for optimizing the design and fabrication of high-performance composite halide perovskite solar cells and demonstrate the potential of the FDQ method as a powerful tool for device modeling and optimization.