<p>Carbon capture and storage (CCS) has the potential to help nations meet their Paris Agreement CO<sub>2</sub> reduction commitments<sup><CitationRef CitationID="CR1">1</CitationRef>,<CitationRef CitationID="CR2">2</CitationRef></sup>. The ability to capture CO<sub>2</sub> within mafic and ultramafic rocks through mineralization of carbon is an example of such a CCS technology<sup><CitationRef CitationID="CR3">3</CitationRef>,<CitationRef CitationID="CR4">4</CitationRef></sup>, but large-scale deployment has yet to be achieved<sup><CitationRef CitationID="CR5">5</CitationRef>,<CitationRef CitationID="CR6">6</CitationRef></sup>. Each geologic environment in the Earth’s crust requires a distinct carbon storage solution. Whereas some regions of the subsurface contain saline aquifers and sedimentary traps suitable for traditional carbon storage through the injection of high-pressure, dense CO<sub>2</sub> below impermeable caprocks, other regions may lack caprocks<sup><CitationRef AdditionalCitationIDS="CR6 CR7 CR8" CitationID="CR5">5</CitationRef>–<CitationRef CitationID="CR9">9</CitationRef></sup>. In these regions, carbon storage is possible through the mineralization of injected water-dissolved CO<sub>2</sub> forming stable carbonate minerals through its reactions with reactive silicate rocks and minerals<sup><CitationRef CitationID="CR6">6</CitationRef>,<CitationRef CitationID="CR10">10</CitationRef>,<CitationRef CitationID="CR11">11</CitationRef></sup>. A notable challenge to applying this process at scale is that it can require 20–50 times or more water than the mass of CO<sub>2</sub> stored<sup><CitationRef CitationID="CR12">12</CitationRef></sup>. Here we report on an industrial-scale pilot project designed to find a carbon disposal solution for western Saudi Arabia. This arid region has large point-source CO<sub>2</sub> emitters, including petroleum refining and desalination facilities, but lacks saline aquifers and sedimentary traps<sup><CitationRef AdditionalCitationIDS="CR14 CR15 CR16" CitationID="CR13">13</CitationRef>–<CitationRef CitationID="CR17">17</CitationRef></sup>. We find that a CO<sub>2</sub> injection approach based on the recirculation of subsurface fluids can eliminate the need for external water. Our results demonstrate the feasibility of carbon mineral storage in regions in which access to water resources may be limited.</p>

错误:搜索内容不能为空,请输入英文关键词
错误:关键词超出字数限制,请精简
高级检索

CO2 subsurface mineral storage by its co-injection with recirculating water

  • Eric H. Oelkers,
  • Serguey Arkadakskiy,
  • Zeyad Ahmed,
  • Noushad Kunnummal,
  • Jakub Fedorik,
  • Massimo Marchesi,
  • Mouadh Addassi,
  • Abdirizak Omar,
  • Niccolo Menegoni,
  • Sigurdur R. Gislason,
  • Grimur Bjornsson,
  • Davide Berno,
  • Thomas Finkbeiner,
  • Abdulkader Afifi,
  • Hussein Hoteit

摘要

Carbon capture and storage (CCS) has the potential to help nations meet their Paris Agreement CO2 reduction commitments1,2. The ability to capture CO2 within mafic and ultramafic rocks through mineralization of carbon is an example of such a CCS technology3,4, but large-scale deployment has yet to be achieved5,6. Each geologic environment in the Earth’s crust requires a distinct carbon storage solution. Whereas some regions of the subsurface contain saline aquifers and sedimentary traps suitable for traditional carbon storage through the injection of high-pressure, dense CO2 below impermeable caprocks, other regions may lack caprocks59. In these regions, carbon storage is possible through the mineralization of injected water-dissolved CO2 forming stable carbonate minerals through its reactions with reactive silicate rocks and minerals6,10,11. A notable challenge to applying this process at scale is that it can require 20–50 times or more water than the mass of CO2 stored12. Here we report on an industrial-scale pilot project designed to find a carbon disposal solution for western Saudi Arabia. This arid region has large point-source CO2 emitters, including petroleum refining and desalination facilities, but lacks saline aquifers and sedimentary traps1317. We find that a CO2 injection approach based on the recirculation of subsurface fluids can eliminate the need for external water. Our results demonstrate the feasibility of carbon mineral storage in regions in which access to water resources may be limited.