<p>Microplastic and nanoplastic particles (MNPs) are pervasive in the atmosphere, yet their direct radiative forcing (DRF) remains poorly constrained. Using a radiative transfer model combined with experimentally derived optical properties and simulated atmospheric distributions, we show that coloured MNPs exhibit strong light absorption, with a mean refractive index of 1.49–0.22<i>i</i> at 550 nm and absorption coefficients 74.8 times higher than those of pristine particles. Atmospheric ageing produces minimal net optical change, as yellowing-induced absorption in white particles is largely offset by bleaching of red ones. Modelled global surface concentrations reach 4.18 MP m<sup>−</sup><sup>3</sup> for microplastics and 3.67 ng m<sup>−</sup><sup>3</sup> for nanoplastics. Resulting simulations yield mean DRF of 0.039 ± 0.019 W m<sup>−</sup><sup>2</sup> for MNPs, equivalent to 16.2% of black carbon forcing. Regional DRF peaks over the North Pacific Subtropical Gyre (~1.34 W m<sup>−</sup><sup>2</sup>), exceeded located black carbon by 4.7-fold, highlighting MNPs as previously unrecognized climate forcing agents.</p>

错误:搜索内容不能为空,请输入英文关键词
错误:关键词超出字数限制,请精简
高级检索

Atmospheric warming contributions from airborne microplastics and nanoplastics

  • Yu Liu,
  • Hongbo Fu,
  • Hongliang Zhang,
  • Yunhang Wang,
  • Rajan K. Chakrabarty,
  • Xiang Tu,
  • Xu Tang,
  • Alexander Laskin,
  • Gregory R. Carmichael,
  • Jianmin Chen,
  • Joseph S. Francisco,
  • Drew T. Shindell

摘要

Microplastic and nanoplastic particles (MNPs) are pervasive in the atmosphere, yet their direct radiative forcing (DRF) remains poorly constrained. Using a radiative transfer model combined with experimentally derived optical properties and simulated atmospheric distributions, we show that coloured MNPs exhibit strong light absorption, with a mean refractive index of 1.49–0.22i at 550 nm and absorption coefficients 74.8 times higher than those of pristine particles. Atmospheric ageing produces minimal net optical change, as yellowing-induced absorption in white particles is largely offset by bleaching of red ones. Modelled global surface concentrations reach 4.18 MP m3 for microplastics and 3.67 ng m3 for nanoplastics. Resulting simulations yield mean DRF of 0.039 ± 0.019 W m2 for MNPs, equivalent to 16.2% of black carbon forcing. Regional DRF peaks over the North Pacific Subtropical Gyre (~1.34 W m2), exceeded located black carbon by 4.7-fold, highlighting MNPs as previously unrecognized climate forcing agents.