<p>Exciton-polaritons – coherently hybridized states of excitons and photons – are instrumental for solid-state nonlinear optics and quantum simulations. To enable engineered polariton energy landscapes and interactions, local control over the particle-like states can be achieved by tuning the properties of the exciton constituent. Monolayer transition metal dichalcogenides stand out in this respect, as they readily allow for a deterministic, flexible and scalable control of excitons, and thus of hybrid exciton-polaritons, via environmental dielectric engineering. Here, we demonstrate the realization of mesoscopic exciton-polariton domains in a structured dielectric exciton environment, and establish an effective long-range exciton hopping in the dispersive regime of cavity-coupling. Our results represent a crucial step toward interacting polaritonic networks and quantum simulations in exciton-polariton lattices based on dielectrically tailored two-dimensional semiconductors.</p>

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Cavity-mediated exciton hopping in a dielectrically engineered polariton system

  • Lukas Husel,
  • Farsane Tabataba-Vakili,
  • Johannes Scherzer,
  • Lukas Krelle,
  • Ismail Bilgin,
  • Samarth Vadia,
  • Kenji Watanabe,
  • Takashi Taniguchi,
  • Iacopo Carusotto,
  • Alexander Högele

摘要

Exciton-polaritons – coherently hybridized states of excitons and photons – are instrumental for solid-state nonlinear optics and quantum simulations. To enable engineered polariton energy landscapes and interactions, local control over the particle-like states can be achieved by tuning the properties of the exciton constituent. Monolayer transition metal dichalcogenides stand out in this respect, as they readily allow for a deterministic, flexible and scalable control of excitons, and thus of hybrid exciton-polaritons, via environmental dielectric engineering. Here, we demonstrate the realization of mesoscopic exciton-polariton domains in a structured dielectric exciton environment, and establish an effective long-range exciton hopping in the dispersive regime of cavity-coupling. Our results represent a crucial step toward interacting polaritonic networks and quantum simulations in exciton-polariton lattices based on dielectrically tailored two-dimensional semiconductors.