<p>Advancements in stone bead technology, particularly in drilling techniques, emerged during the Indus Valley (Harappan) civilization. Long-constricted cylindrical drill bits, made from a unique stone called Ernestite, were a distinctive feature of this culture. The origin of Ernestite remains uncertain, as it has no known natural analog and its synthesis process is poorly understood. This study presents a mineralogical and geochemical investigation of Ernestite stones and drill bits from multiple Harappan and contemporaneous sites in Gujarat, India, to uncover their origin. The ⁸⁷Sr/⁸⁶Sr and ε_Nd(0) of the drill bits overlap with those of the Ernestite stones, confirming their genetic relationship. The texture and presence of pseudo-mullite (SiO₂ &gt; 40 wt%) with high Al-Ti-bearing hematite suggest that Ernestites are synthetic, created through a sintering process at ~1100 °C. An abundance of sand to silt-sized detrital quartz, along with Fe-Ti-Zr-rich minerals, indicates the use of unevenly powdered sandstones and laterites as raw materials, with geochemical ties to regional sources.</p>