<p>The growing global water crisis necessitates innovative solutions that are both cost-effective and environmentally sustainable. Atmospheric water harvesting (AWH) has emerged as a promising avenue of research to address this pressing challenge. Here, we present a novel approach that re-purposes low-value petroleum feedstocks for AWH through their conversion to porous carbon (PC). Utilizing a potassium carbonate-assisted carbonization process, we develop PC from heavy and light cycle oils, and vacuum residue. While all sources yield materials with near superhydrophilic surfaces, only the cycle oils produce PC with high surface area and micoporous architectures. These engineered carbons demonstrate great water adsorption capacities of up to 23 wt% at 60% relative humidity (RH), surpassing commercially available carbon materials.</p>

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Leveraging petroleum-derived carbon for atmospheric water harvesting

  • Wala Algozeeb,
  • Ahmed Owais,
  • Qasim Saleem,
  • Noha Al-Shihri,
  • Emad Al-Shafie,
  • Hendrik Muller,
  • Nadrah Alawani,
  • Abdulkarim Makki,
  • Hasan Al-Tarouti,
  • Amer Al Tuwailib,
  • Ahmed AlAsseel,
  • Ibrahim Al-Zahrani

摘要

The growing global water crisis necessitates innovative solutions that are both cost-effective and environmentally sustainable. Atmospheric water harvesting (AWH) has emerged as a promising avenue of research to address this pressing challenge. Here, we present a novel approach that re-purposes low-value petroleum feedstocks for AWH through their conversion to porous carbon (PC). Utilizing a potassium carbonate-assisted carbonization process, we develop PC from heavy and light cycle oils, and vacuum residue. While all sources yield materials with near superhydrophilic surfaces, only the cycle oils produce PC with high surface area and micoporous architectures. These engineered carbons demonstrate great water adsorption capacities of up to 23 wt% at 60% relative humidity (RH), surpassing commercially available carbon materials.