<p>Perovskites have attracted widespread attention for laser applications due to their excellent optoelectronic properties. However, perovskite lasers typically exhibit a wavelength shift as pump density increases. Here, we report a pump-induced wavelength shift-free laser achieved using a perovskite nanoplatelet with mixed orthorhombic and tetragonal phase. At 293 K, the tetragonal-phase perovskite nanoplatelet laser exhibits a blue shift of ~0.4 nm µJ<sup>−1</sup> cm<sup>2</sup> with increasing pump density. In contrast, at 80 K, the orthorhombic-phase perovskite nanoplatelet laser exhibits a red shift of ~1 nm µJ<sup>−1</sup> cm<sup>2</sup>. By stabilizing the perovskite nanoplatelet in a mixed orthorhombic-tetragonal phase at 163 K, the pump induced wavelength shifts are completely suppressed, resulting in a wavelength-stable laser. Additionally, the lasing threshold decreases from 18.4 µJ cm<sup>−2</sup> at room temperature to 4.5 µJ cm<sup>−2</sup> at 163 K. This study presents a promising strategy for achieving pump-insensitive wavelength stability in micro/nano lasers.</p>

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Stable-wavelength perovskite nanoplatelet laser via mixed-phase engineering

  • Guohui Li,
  • Yulong Ji,
  • Ruofan Zhao,
  • Lin Xue,
  • Ye Zhang,
  • Kaibo Zheng,
  • Yanxia Cui

摘要

Perovskites have attracted widespread attention for laser applications due to their excellent optoelectronic properties. However, perovskite lasers typically exhibit a wavelength shift as pump density increases. Here, we report a pump-induced wavelength shift-free laser achieved using a perovskite nanoplatelet with mixed orthorhombic and tetragonal phase. At 293 K, the tetragonal-phase perovskite nanoplatelet laser exhibits a blue shift of ~0.4 nm µJ−1 cm2 with increasing pump density. In contrast, at 80 K, the orthorhombic-phase perovskite nanoplatelet laser exhibits a red shift of ~1 nm µJ−1 cm2. By stabilizing the perovskite nanoplatelet in a mixed orthorhombic-tetragonal phase at 163 K, the pump induced wavelength shifts are completely suppressed, resulting in a wavelength-stable laser. Additionally, the lasing threshold decreases from 18.4 µJ cm−2 at room temperature to 4.5 µJ cm−2 at 163 K. This study presents a promising strategy for achieving pump-insensitive wavelength stability in micro/nano lasers.