<p>The CaO-Na<sub>2</sub>O-Al<sub>2</sub>O<sub>3</sub>-B<sub>2</sub>O<sub>3</sub>-Ho<sub>2</sub>O<sub>3</sub> glasses (0 ≤ x ≤ 2&#xa0;mol%) were fabricated via melt quenching technique. Comprehensive characterization revealed an increase in density, molar volume, and refractive index with rising Ho<sup>3+</sup> ion concentration. Optical absorption spectra analysis yielded Judd–Ofelt parameters: Ω<sub>2</sub> = 6.4268 × 10<sup>−20</sup>&#xa0;cm<sup>2</sup>, Ω<sub>4</sub> = 2.7468 × 10<sup>−20</sup>&#xa0;cm<sup>2</sup>, and Ω<sub>6</sub> = 2.5888 × 10<sup>−20</sup>&#xa0;cm<sup>2</sup>. These results indicate promising optical properties for CaNaAlB glass doped with 0.1&#xa0;mol% Ho<sub>2</sub>O<sub>3</sub>. Experimental and calculated branching ratios for <sup>5</sup>F<sub>4</sub> → <sup>5</sup>I<sub>8</sub> transition is recorded to be 0.64 and 0.82 respectively. The stimulated emission cross-section for NaCaAlB glasses was 4434&#xa0;s<sup>−1</sup>, while the total radiative transition probability was 5294.48&#xa0;s<sup>−1</sup>. Chromaticity coordinates for NaCaAlB glasses doped with Ho<sup>3+</sup> ions were calculated, confirming their potential for green lighting and eye safe laser&#xa0;applications.</p>

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A spectroscopic investigations of Ho3+ doped CaO-Na2O-Al2O3-B2O3 glass for green lighting and eye-safe lasers applications

  • I. Khan,
  • M. Shoaib,
  • Abdullah M. S. Alhuthali,
  • Rustem R. Zairov,
  • Alexander Yu. Kopylov,
  • I. Ullah,
  • Ahmad A. Ifseisi,
  • Mohamed E. Assal,
  • G. Rooh,
  • N. Chanthima,
  • N. Intachai,
  • S. Kothan,
  • Xiao Lixian,
  • He YongTai,
  • J. Kaewkhao

摘要

The CaO-Na2O-Al2O3-B2O3-Ho2O3 glasses (0 ≤ x ≤ 2 mol%) were fabricated via melt quenching technique. Comprehensive characterization revealed an increase in density, molar volume, and refractive index with rising Ho3+ ion concentration. Optical absorption spectra analysis yielded Judd–Ofelt parameters: Ω2 = 6.4268 × 10−20 cm2, Ω4 = 2.7468 × 10−20 cm2, and Ω6 = 2.5888 × 10−20 cm2. These results indicate promising optical properties for CaNaAlB glass doped with 0.1 mol% Ho2O3. Experimental and calculated branching ratios for 5F4 → 5I8 transition is recorded to be 0.64 and 0.82 respectively. The stimulated emission cross-section for NaCaAlB glasses was 4434 s−1, while the total radiative transition probability was 5294.48 s−1. Chromaticity coordinates for NaCaAlB glasses doped with Ho3+ ions were calculated, confirming their potential for green lighting and eye safe laser applications.