Abstract <p>Functional signal conversion devices are critical components of next-generation intelligent systems, driving an urgent demand for novel sensing materials and functionalities to enable advanced applications in intelligent robotics and human–machine interfaces. In this work, we present a quantum dot light-emitting diode (QLED) array based on a newly developed signal conversion functional material 20% Gd-doped CeO<sub>2−<i>x</i></sub> (CGO). Under pressure and electric field induction, the oxygen vacancy dynamics in CGO were modulated, resulting in macroscopic polarization charges, reflecting the mechanical force-electrical response effect. The QLED pixel emission intensity was controlled by external pressure, achieving a remarkable 1000% enhancement at 1.8&#xa0;GPa. Combined with resolution-tunable Si MWs array, mapping of 2D pressure distribution on external objects with optical signals was realized. This work extends the force-electrical-optical signal conversion mechanism to centrosymmetric cubic fluorite materials, overcoming the traditional limitations of piezo-phototronic devices that rely on specific crystal symmetries, and provides new avenues for the development of the next-generation smart sensing.</p> Graphical abstract <p>A flexible QLED array with the ability to modulate the intensity of pixels light emission through mechanical stimulation is designed in this paper. The device expands the application of force-electro-optical coupling devices in the field of tactile sensing and provides new ideas for the development of sensing materials and functional devices.</p>

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Flexible QLED array with mechanical force modulation of electroluminescence intensity

  • Ye-Pei Mo,
  • Yue Liu,
  • Li Zhang,
  • Xin-Gang Pan,
  • Zhi-Wei Fu,
  • Wen-Chao Gao,
  • Rong-Rong Bao,
  • Cao-Feng Pan

摘要

Abstract

Functional signal conversion devices are critical components of next-generation intelligent systems, driving an urgent demand for novel sensing materials and functionalities to enable advanced applications in intelligent robotics and human–machine interfaces. In this work, we present a quantum dot light-emitting diode (QLED) array based on a newly developed signal conversion functional material 20% Gd-doped CeO2−x (CGO). Under pressure and electric field induction, the oxygen vacancy dynamics in CGO were modulated, resulting in macroscopic polarization charges, reflecting the mechanical force-electrical response effect. The QLED pixel emission intensity was controlled by external pressure, achieving a remarkable 1000% enhancement at 1.8 GPa. Combined with resolution-tunable Si MWs array, mapping of 2D pressure distribution on external objects with optical signals was realized. This work extends the force-electrical-optical signal conversion mechanism to centrosymmetric cubic fluorite materials, overcoming the traditional limitations of piezo-phototronic devices that rely on specific crystal symmetries, and provides new avenues for the development of the next-generation smart sensing.

Graphical abstract

A flexible QLED array with the ability to modulate the intensity of pixels light emission through mechanical stimulation is designed in this paper. The device expands the application of force-electro-optical coupling devices in the field of tactile sensing and provides new ideas for the development of sensing materials and functional devices.