Scholarlink

<p>Impulsive stimulated Raman spectroscopy using a chirped broadband probe pulse (broadband ISRS) has attracted significant attention due to its numerous advantages over spontaneous Raman spectroscopy, stimulated Raman spectroscopy (SRS), and ISRS with a probe pulse spectrally degenerate with the Raman pump pulse (degenerate ISRS). In this article, we present a non-mathematical perspective on ISRS, covering its machinery and applications. In particular, we demonstrate how broadband ISRS can extract a tiny Raman signal from a strong fluorescence background, both having the same Stokes shift.</p> Graphical abstract <p>The usefulness of broadband impulsive stimulated Raman spectroscopy over conventional approaches for isolating a feeble Raman signal with the same Stokes shift as a strong fluorescence background is demonstrated.</p>

错误：搜索内容不能为空，请输入英文关键词
错误：关键词超出字数限制，请精简
高级检索

Broadband impulsive stimulated Raman spectroscopy: A fluorescence-background-free alternative to conventional Raman spectroscopy

  • 期刊论文

  • 发表日期：

    2026年6月15日

查看全文
  • Shaina Dhamija,
  • Garima Bhutani,
  • Arijit K De

摘要

Impulsive stimulated Raman spectroscopy using a chirped broadband probe pulse (broadband ISRS) has attracted significant attention due to its numerous advantages over spontaneous Raman spectroscopy, stimulated Raman spectroscopy (SRS), and ISRS with a probe pulse spectrally degenerate with the Raman pump pulse (degenerate ISRS). In this article, we present a non-mathematical perspective on ISRS, covering its machinery and applications. In particular, we demonstrate how broadband ISRS can extract a tiny Raman signal from a strong fluorescence background, both having the same Stokes shift.

Graphical abstract

The usefulness of broadband impulsive stimulated Raman spectroscopy over conventional approaches for isolating a feeble Raman signal with the same Stokes shift as a strong fluorescence background is demonstrated.