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<p>The urgent demand for high-performance and sustainable energy storage solutions necessitates the development of advanced electrolytes with superior electrochemical properties. Hybrid lithium electrolytes, which integrate the advantages of inorganic and organic ionic conductors, have emerged as promising candidates for next-generation energy storage devices. This review presents a comprehensive bibliometric analysis of 1569 research articles from 2019 to 2024, sourced from Scopus and Web of Science (WOS) databases, highlighting the rising research focus on hybrid electrolytes. Key material properties such as wide electrochemical windows, thermal and chemical stability, low toxicity, and reduced volatility are critical for enhancing battery performance. The discussion encompasses recent advancements in solid-state, polymer, and hybrid electrolytes, emphasizing their role in improving energy density, cycling stability, and safety. Furthermore, this study examines the challenges associated with hybrid electrolytes, including ionic conductivity limitations, interfacial compatibility, and scalability for industrial applications. The integration of novel materials such as NASICON-type ceramics, perovskites, sulfides, and garnet-based electrolytes is explored for their potential to revolutionize lithium-ion battery technologies. By bridging the gap between fundamental research and practical implementation, this review provides insights into the future directions of hybrid electrolytes, paving the way for more efficient and sustainable energy storage systems.</p> Graphical Abstract <p></p>

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Hybrid Lithium Electrolytes as Potential Electrolytes for Energy Storage Devices: A Pathway to Sustainable and High-Efficiency Solutions

  • 期刊论文

  • 发表日期：

    2025年7月29日

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  • Chitra Sharma,
  • Harpreet Kaur,
  • Abhinay Thakur,
  • Ramesh Chand Thakur,
  • Harmanjit Singh Dosanjh

摘要

The urgent demand for high-performance and sustainable energy storage solutions necessitates the development of advanced electrolytes with superior electrochemical properties. Hybrid lithium electrolytes, which integrate the advantages of inorganic and organic ionic conductors, have emerged as promising candidates for next-generation energy storage devices. This review presents a comprehensive bibliometric analysis of 1569 research articles from 2019 to 2024, sourced from Scopus and Web of Science (WOS) databases, highlighting the rising research focus on hybrid electrolytes. Key material properties such as wide electrochemical windows, thermal and chemical stability, low toxicity, and reduced volatility are critical for enhancing battery performance. The discussion encompasses recent advancements in solid-state, polymer, and hybrid electrolytes, emphasizing their role in improving energy density, cycling stability, and safety. Furthermore, this study examines the challenges associated with hybrid electrolytes, including ionic conductivity limitations, interfacial compatibility, and scalability for industrial applications. The integration of novel materials such as NASICON-type ceramics, perovskites, sulfides, and garnet-based electrolytes is explored for their potential to revolutionize lithium-ion battery technologies. By bridging the gap between fundamental research and practical implementation, this review provides insights into the future directions of hybrid electrolytes, paving the way for more efficient and sustainable energy storage systems.

Graphical Abstract