<p>Tb-doped LiYSiO<sub>4</sub> was fabricated and evaluated as thermoluminescent (TL) materials for thermal neutron detection. Tb was introduced as a luminescent center. Because neutron fields generally contain gamma-rays, a subtraction method was employed to enable neutron–gamma discrimination, utilizing the difference in TL responses between <sup>n</sup>Li (natural isotopic abundance) and <sup>6</sup>Li-enriched samples, due to the high neutron capture sensitivity of <sup>6</sup>Li. After X-ray irradiation, both samples exhibited similar TL glow curves, which indicate their comparable X-ray and gamma-ray responses. After neutron irradiation, the <sup>6</sup>Li-enriched sample showed significantly higher TL intensity than the <sup>n</sup>Li sample, and the observed difference was attributed to neutron-induced TL signals. Thermal neutron fluence was measurable within the investigated range of 10<sup>5</sup>–10<sup>9</sup> neutrons cm<sup>−2</sup> with an estimated detection limit of 6.2 × 10<sup>4</sup> neutrons cm<sup>–2</sup>, which is comparable to that of commercial neutron dosimeter pairs such as TLD-600/TLD-700.</p>

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Neutron-induced thermoluminescence properties of Tb3+-doped LiYSiO4 ceramics

  • Yuta Hiramatsu,
  • Genichiro Wakabayashi,
  • Masanori Koshimizu

摘要

Tb-doped LiYSiO4 was fabricated and evaluated as thermoluminescent (TL) materials for thermal neutron detection. Tb was introduced as a luminescent center. Because neutron fields generally contain gamma-rays, a subtraction method was employed to enable neutron–gamma discrimination, utilizing the difference in TL responses between nLi (natural isotopic abundance) and 6Li-enriched samples, due to the high neutron capture sensitivity of 6Li. After X-ray irradiation, both samples exhibited similar TL glow curves, which indicate their comparable X-ray and gamma-ray responses. After neutron irradiation, the 6Li-enriched sample showed significantly higher TL intensity than the nLi sample, and the observed difference was attributed to neutron-induced TL signals. Thermal neutron fluence was measurable within the investigated range of 105–109 neutrons cm−2 with an estimated detection limit of 6.2 × 104 neutrons cm–2, which is comparable to that of commercial neutron dosimeter pairs such as TLD-600/TLD-700.