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<p>The single crystal of 2-Amino-4,6-dimethylpyrimidinium hydrogen sulphate (2DPHS) has a distinctive structural composition that offers several potential benefits, particularly in the fields of materials science and chemistry. This paper emphasizes the growth of defect-free, high-quality, measured-size 2DPHS single crystals via a solution growth process. The grown crystal was investigated for its structural, optical, thermal, and third-order nonlinear optical (NLO) properties. “The XRD results confirm that 2DPHS crystallizes in a monoclinic structure. FTIR analysis verifies the presence of the required functional groups in the 2DPHS single crystal. An extensive discussion on the crystal’s linear and third-order nonlinear optical characteristics is presented in this work. The substantial photocurrent output exhibited by the 2DPHS single crystal highlights its potential application in various optical devices, including light-emitting diodes (LEDs), lasers, and optical modulators. The modified growth conditions enhance the optical properties of the grown crystals compared to our previous reports.</p>

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Experimental investigation on the structural and physio-chemical properties of 2-amino-4,6-dimethyl-pyrimidinium hydrogen sulphate (2dphs) single crystal

  • 期刊论文

  • 发表日期：

    2025年5月30日

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  • T. Rasappan,
  • C. Besky Job,
  • B. Sahaya Infant Lasalle,
  • C. Justin Dhanraj,
  • Muthu Senthil Pandian,
  • P. Ramasamy,
  • P. Selvarajan

摘要

The single crystal of 2-Amino-4,6-dimethylpyrimidinium hydrogen sulphate (2DPHS) has a distinctive structural composition that offers several potential benefits, particularly in the fields of materials science and chemistry. This paper emphasizes the growth of defect-free, high-quality, measured-size 2DPHS single crystals via a solution growth process. The grown crystal was investigated for its structural, optical, thermal, and third-order nonlinear optical (NLO) properties. “The XRD results confirm that 2DPHS crystallizes in a monoclinic structure. FTIR analysis verifies the presence of the required functional groups in the 2DPHS single crystal. An extensive discussion on the crystal’s linear and third-order nonlinear optical characteristics is presented in this work. The substantial photocurrent output exhibited by the 2DPHS single crystal highlights its potential application in various optical devices, including light-emitting diodes (LEDs), lasers, and optical modulators. The modified growth conditions enhance the optical properties of the grown crystals compared to our previous reports.