Evaluation of radon surface exhalation rates in the soil and its transport mechanisms around Chakrata region of Garhwal-Himalayan Terrain, India
摘要
Radon, a naturally occurring radioactive gas produced from the decay of uranium in the subsurface, migrates upward through soil by diffusion and advection before being released into the atmosphere. As the second leading cause of lung cancer after smoking, understanding its behavior in the near-surface environment is essential for assessing environmental radiation risks. This study investigates depth-wise radon concentrations in soil gas, surface exhalation rates, and transport parameters in the soil of Chakrata region, Garhwal Himalaya, India. Radon measurements were performed using a portable Smart RnDuo monitor at depths (Z) of 15, 30, and 45 cm. Soil-gas radon concentrations ranges from 237 to 6540 Bq m−3 at 15 cm, 854 to 7831 Bq m−3 at 30 cm, and 1020 to 8540 Bq m−3 at 45 cm, indicating a systematic increase with depth. Surface exhalation rates varies between 1.25 and 16.19 Bq m−2 h−1, with a mean value of 6.42 Bq m−2 h−1, respectively. Radon transport parameters were derived using Fick’s diffusion model, resulting in average values of 0.49 m for diffusion length (ls) and 0.002 m2s−1 for diffusion coefficient (Ds). Spearman’s rank correlation analysis revealed that surface radon exhalation and diffusion parameters exhibit strong correlations. These findings provide baseline information on radon mobility and soil-gas dynamics in the region and will support future radon hazard assessment and environmental monitoring efforts in the Chakrata area of the Lesser Indian Himalaya.