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<p>Although the use of biochar as an adsorbent for the removal of various pollutants from wastewater is well established, the use of biochar/modified biochar for the scavenging of antibiotics from aqueous media in the Fenton-like system receives less attention. The highest kasugamycin (KSM) adsorption capacity (5.0&#xa0;mg&#xa0;g<sup>−1</sup>) was obtained from the pristine biochar at the lowest initial pH of 3 in Fenton-like system. The Fenton-like system improved the KSM adsorption capacity of pristine biochar by 222.2%, 169.9%, and 159.9% at 25&#xa0;°C, 35&#xa0;°C, and 45&#xa0;°C comparing to control, respectively, and it also increased adsorption capacity by 97.4%, 63.8%, and 56.8% comparing to modified biochar. The amounts of biochar applied and the Fenton-like system affected KSM mineralization and degradation. The KSM degradation products had a significant amount of small molecular organic matter (m/z 384) and a tetrahydropyran structure that was difficult to degrade. The highly efficient degradation of KSM in Fenton-like system can be attributed to the generation of large amounts of hydroxyl radical (·OH) and functional groups (C=C, C=O, etc.).</p>

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Evaluation of Fenton-like reaction for sorption and degradation of kasugamycin in the presence of biochar

  • 期刊论文

  • 发表日期：

    2025年1月15日

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  • Wei Zhang,
  • Liqiang Cui,
  • Jingwen Ma,
  • Shuyan Cui,
  • Guixiang Quan,
  • Jinlong Yan,
  • Fengfeng Sui,
  • Hui Wang,
  • Kiran Hina,
  • Qaiser Hussain

摘要

Although the use of biochar as an adsorbent for the removal of various pollutants from wastewater is well established, the use of biochar/modified biochar for the scavenging of antibiotics from aqueous media in the Fenton-like system receives less attention. The highest kasugamycin (KSM) adsorption capacity (5.0 mg g−1) was obtained from the pristine biochar at the lowest initial pH of 3 in Fenton-like system. The Fenton-like system improved the KSM adsorption capacity of pristine biochar by 222.2%, 169.9%, and 159.9% at 25 °C, 35 °C, and 45 °C comparing to control, respectively, and it also increased adsorption capacity by 97.4%, 63.8%, and 56.8% comparing to modified biochar. The amounts of biochar applied and the Fenton-like system affected KSM mineralization and degradation. The KSM degradation products had a significant amount of small molecular organic matter (m/z 384) and a tetrahydropyran structure that was difficult to degrade. The highly efficient degradation of KSM in Fenton-like system can be attributed to the generation of large amounts of hydroxyl radical (·OH) and functional groups (C=C, C=O, etc.).